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Microscopic description of fission in superheavy nuclei with the parametrization D1M ∗ of the Gogny energy density functional

Authors

R. Rodríguez-Guzmán, Y. M. Humadi and L. M. Robledo

Journal Paper

https://doi.org/10.1140/epja/s10050-020-00051-w

Publisher URL

https://link.springer.com/

Publication date

February 2020

The constrained Hartree–Fock–Bogoliubov approximation, based on the recent parametrization D1M of the Gogny energy density functional, is used to describe fission in 435 superheavy nuclei. The Gogny-D1M parametrization is benchmarked against available experimental data on inner and second barrier heights, excitation energies of the fission isomers and half-lives in a selected set of Pu, Cm, Cf, Fm, No, Rf, Sg, Hs and Fl nuclei. Results are also compared with those obtained with the Gogny-D1M energy density functional. A detailed study of the minimal energy fission paths is carried out for isotopic chains with atomic numbers 100 ≤ Z≤ 126 including very neutron-rich sectors up to around 4 MeV from the two-neutron driplines. Single-particle energies, ground state deformations, pairing correlations, two-nucleon separation energies and barrier heights are also discussed. In addition to fission paths, the constrained Hartree–Fock–Bogoliubov framework provides collective masses and zero-point quantum rotational and vibrational energies. Those quantities are building blocks within the Wentzel–Kramer–Brillouin formalism employed to evaluate the systematic of the spontaneous fission half-lives tSF. The competition between spontaneous fission and α-decay is studied, through the computation of the α-decay half-lives tα using a parametrization of the Viola–Seaborg formula. From the comparison with the available experimental data and the results obtained with other theoretical approaches, it is concluded that D1M represents a reasonable starting point to describe fission in heavy and superheavy nuclei.